By Akihiko Iwashita, Haruyuki Makio (auth.), Juan CAMPORA, Giuliano GIAMBASTIANI (eds.)

ISBN-10: 9400706952

ISBN-13: 9789400706958

Olefin Upgrading Catalysis by means of Nitrogen-based steel Complexes II: cutting-edge and views presents a serious overview of the cutting-edge advancements in industrially suitable techniques attached to effective and selective olefin upgrading. particular realization is dedicated to catalysts containing imine- and amine-based ligands.

All the chapters during this e-book were designed to supply a scientific account of the sizeable volume of knowledge on hand for this kind of catalyst in addition to to focus on the criteria that finally keep an eye on the catalyst’s functionality and productiveness. A finished landscape of catalyst precursors is gifted, spanning from workforce 10

α-diimine complexes and iron and cobalt 2,6-bis(imino)pyridine derivatives, to vanadium, chromium, titanium, zirconium and lanthanide complexes supported by way of nitrogen-containing ligands. The authors of this collective paintings are presently focused on the improvement of imine-based catalysts for effective and selective olefin upgrading and the vast majority of them have devoted so much in their medical occupation to this crucial box. In penning this ebook, their significant aim is to move as many principles and reports as attainable to the worldwide viewers of scientists engaged during this region of research.

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Extra info for Olefin Upgrading Catalysis by Nitrogen-based Metal Complexes II: State of the art and Perspectives

Example text

However, Fujita and Coates independently revealed that Ti–FI catalysts upon activation with MAO unexpectedly displayed moderate to extremely high syndioselectivity toward propylene polymerizations, which is mediated via a chain-end control mechanism [50, 80]. Significantly, propylene polymerizations with Ti–FI catalysts having at least one ortho-fluorine on the N-aryl R1 groups exhibit robust living polymerization behavior in the same way as seen for ethylene polymerization with the same catalysts.

Well-controlled living polymerizations allowed for systematic investigations on thermal and mechanical properties of these diblock copolymers. Tensile tests on the diblock copolymer exhibited better extensibility and toughness in comparison to the corresponding random copolymer and the polymer blend. Scientists at Dow Chemical Co. achieved production of olefin multi-block copolymers using two different catalysts capable of a catalytic chain growth on zinc [116–118]. In catalytic chain growth, a growing polymer chain on a transition metal catalyst is transferred to a main group metal (zinc in this case) via transmetallation, which is transferred back to another transition metal in a reversible manner.

Mazzeo M, Strianese M, Lamberti M, Santoriello I, Pellecchia C (2006) Macromolecules 39:7812 90. Corradini P, Guerra G, Cavallo L (2004) Acc Chem Res 37:231 91. Saito J, Onda M, Matsui S, Mitani M, Furuyama R, Tanaka H, Fujita T (2002) Macromol Rapid Commun 23:1118 92. Prasad AV, Makio H, Saito J, Onda M, Fujita T (2004) Chem Lett 33:250 93. Mason AF, Coates GW (2004) J Am Chem Soc 126:16326 94. Edson JB, Wang Z, Kramer EJ, Coates GW (2008) J Am Chem Soc 130:4968 95. Saito J, Suzuki Y, Fujita T (2003) Chem Lett 32:236 96.

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Olefin Upgrading Catalysis by Nitrogen-based Metal Complexes II: State of the art and Perspectives by Akihiko Iwashita, Haruyuki Makio (auth.), Juan CAMPORA, Giuliano GIAMBASTIANI (eds.)


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